Ultrafast nanooptics
Theory of spatio-temporally resolved optical dynamics in hybrid-nanostructures (Richter, Schmidt)
Inhomogeneous spatio-temporal excitation of elementary excitations can be used to study the dynamics of transport phenomena within hybrid nanostructures and between their constituents.
In particular, we focus on the theoretical description of
- the femtosecond excitation transfer on a nanometer scale in metal and semiconductor-hybrid structures, as well as
- the internal dynamics of compound elementary excitations.
We aim at:
- a self-consistent description of optically induced excitation transfer in hybrid nanostructures,
- the manipulation of internal motion of elementary excitations by spatially localized fields, and
- proposals for new spatially resolved spectroscopic methods to observe information on the internal dynamics in hybrid structures.
Therefore,
- we address excitation transfer between the constituents of hybrids, examples are:
coupled circular silver islands and semiconductor wires including carbon nanotubes, silver/gold nanoantennas coupled to quantum dots, including single quantum dots placed in an inverse bowtie structure, coupled quantum dots near a silver/gold nanostructure. - we address the question to what extent internal degrees of freedom (relative motion of a compound elementary excitation) in spatially extended structures can be manipulated by nanoscale spatial gradients of the applied optical fields.
Typical examples are:
electron-hole distributions in bound exciton states,
electron/exciton-phonon clouds in polarons. - On top of these microscopic material studies, coherent spatially resolved nonlinear spectroscopic signals will be applied to these systems.
Publications
Numerical solution of nonlocal hydrodynamic Drude model for arbitrary shaped nano-plasmonic structures using finite elements method
arXiv:1201.1527v1 (2012)
Tunable Plasmon Coupling in Distance-Controlled Gold Nanoparticles
Langmuir DOI:10.1021/la3001575 (2012)
Combining nanooptical fields and coherent spectroscopy on systems with delocalized excitons
Proc. SPIE 8260 (2012) 82601V
Induced surface enhancement in coral Pt island films attached to Ag electrodes
Langmuir DOI: 10.1021/la205139g (2012)
Quantum state tomography with nanooptical fields
arXiv:1201.1765v1 (2012)
Ultrafast nonlinear spectroscopy with spatially confined fields
AIP Conf. Proc. 1398 (2011) 94
Finite element method for accurate 3D simulation of plasmonic waveguides.
Proc. SPIE 7604 (2010) 76040F
Spatiotemporal dynamics of optically generated electron-hole excitations in single-walled carbon nanotubes
Phys. Rev. B 81 (2010) 035414